By Martin R. Tant, Anita J. Hill
content material: The constitution and houses of glassy polymers : an outline / Anita J. Hill and Martin R. Tant --
using configurational entropy to derive the kinetic houses of polymer glasses / Edmund A. Di Marzio --
Entropy, landscapes, and fragility in beverages and polymers, and the [delta]Cp [excess warmth means] challenge / C.A. Angell --
Dynamic houses of polymer melts above the glass transition : Monte Carlo simulation effects / Jörg Baschnagel --
The thermal glass transition past the time catch / K.-P. Bohn and J.K. Krüger --
Dynamic Monte Carlo simulation and dielectric measurements of the impact of pore dimension on glass transition temperature and the kingdom of the glass / N. Haralampus, J.P. Northrop, C. Scordalakes, E. Ashmore, W. Martin, D. Kranbuehl, and P.H. Verdier --
Temperature-modulated calorimetry of the frequency dependence of the glass transition of poly(ethylene terephthalate) and polystyrene / Bernhard Wunderlich and Iwao Okazaki --
Polymer glasses : thermodynamic and relaxational elements / Robert Simha --
Structural rest and fragility of glass-forming miscible blends composed of atactic polystyrene and poly(2,6-dimethyl-1,4-phenylene oxide) / Christopher G. Robertson and Garth L. Wilkes --
Dielectric spectroscopy of bisphenol-A polycarbonate and a few of its blends / G.J. Pratt and M.J.A. Smith --
actual getting older close to the beta transition of a poly(amide-imide) / George J. Dallas, Thomas C. Ward, James Rancourt, and Mia Siochi --
Low-temperature leisure of polymers probed by way of photochemical gap burning / Shinjiro Machida, Satomi Tanaka, Kazuyuki Horie, and Binyao Li --
becoming differential scanning calorimetry heating curves for polyetherimide utilizing a version of structural restoration / Sindee L. Simon --
The physics of glassy polycarbonate : superposability and quantity restoration / Paul A. O'Connell, Carl R. Schultheisz, and Gregory B. McKenna --
Polymer-polymer miscibility investigated through temperature modulated differential scanning calorimetry / G.O.R. Alberda van Ekenstein, G. ten Brinke, and T.S. Ellis --
actual getting older in PMMA investigated utilizing positron annihilation, dielectric rest, and dynamic mechanical thermal research / William J. Davis and Richard A. Pethrick --
Craze initiation and failure in glassy poly(ethylene terephthalate) : the consequences of actual getting older with and with no publicity to chemical environments / Martin R. Tant, E.J. Moskala, M.K. Jank, T.J. Pecorini, and Anita J. Hill --
Transitions, homes, and molecular mobility in the course of therapy of thermosetting resins / Jakob Lange, Roman Ekelöf, Nigel A. St. John, and Graeme A. George --
A dynamic probe of tribological methods at metal-polymer interfaces : temporary present iteration / J.T. Dickinson, L. Scudiero, and S.C. Langford --
The impression of orientation by way of sturdy nation procedures at the amorphous areas in poly(vinyl alcohol) and excessive density poly(ethylene) / Anita J. Hill, T.J. Bastow, and R.M. Hodge --
unfastened quantity and delivery houses of barrier and membrane polymers / B.D. Freeman and Anita J. Hill --
The segmental movement and fuel permeability of glassy polymer poly(1-trimethylsilyl-1-propyne) membranes / T. Nakagawa, T. Watanabe, and ok. Nagai --
emptiness spectroscopy of polymers utilizing positronium / Yasuo Ito --
Subnanometer gap homes of cellulose studied by means of positron annihilation lifetime spectroscopy / H. Cao, J.-P. Yuan, Y.C. Jean, A. Pekarovicova, and R.A. Venditti --
Ionic conductivity in glassy PVOH-lithium salt platforms / M. Forsyth, H.A. each, F. Zhou, and D.R. MacFarlane --
Oxygen delivery via electronically conductive polyanilines / Yong Soo Kang, Hyuck Jai Lee, Jina Namgoong, Heung Cho Ko, Hoosung Lee, Bumsuk Jung, and Un younger Kim --
Xenon-129 NMR as a probe of polymer sorption websites : a brand new view of constitution and delivery / J.M. Koons, W.-Y. Wen, P.T. Inglefield, and A.A. Jones --
Dissolution mechanism of glassy polymers : a molecular research / B. Narasimhan and N.A. Peppas --
gasoline barrier and thermal houses of (alkylsulfonyl)methyl-substituted poly(oxyalkylene)s / Jong-Chan Lee, Morton H. Litt, and Charles E. Rogers.
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Sci. 1983, 36, 1413. [15] Gujrati, P. ; Goldstein, M . J. Chem. Phys. 1981, 74, 2596. [16] Foreman, K. ; Freed, K. F. J. Chem. Phys. 1997, 106, 7422; Ibid, In press. ; Paul, W. J. Poly Sci. Pt. ; Binder, K. Phys. Rev. Ε 1996, 54, 1535. [18] Baumgartner, A. J. Phys. 1984, A17, L975 has, through computer modeling, shown strong spatial variation in the orientation order parameter for rigid rod systems. His J. Physique Lett. 1985 46, L659 paper strongly implies that global order parameters will not give a correct view of liquid crystals.
Ch002 c c c 1 c p c C =«/T pc S =a(l/T -1/T) -> c (8) 2 G = -Κ -α(Τ/Τ -1) +aLn(T/T ), T <£T (9a) G = -K, T As with the increase of T , most of the effect is obtained with the first few repeat unit additions. The relation is shown in Figure 3. However the chain length of polymers has generally been found not to affect their fragilities (27,28) (though there is some recent conflict from different estimates in the case of polystyrene (31,32)). Clearly, though, the correlation between A C and fragility seen in the inorganic ionic (33), and covalent (34) network polymers does not hold for carbon chain polymers (in which the in-chain bonds are inviolable).